Let
$\mathcal{E}=\left\{e_1,e_2,e_3\right\}$
be our canonical base. With this base, transormation T has representation
$T=\left(
\begin{array}{ccc}
3 & 1 & 0 \\
1 & 0 & 1 \\
1 & 0 & -1 \\
\end{array}
\right)$.
Now we have got a new base:
$\mathcal{F}=\left\{e_1,e_1+e_2,e_1+e_2+e_3\right\}$.
Let
$M_{\mathcal{F}}=\left(
\begin{array}{ccc}
1 & 1 & 1 \\
0 & 1 & 1 \\
0 & 0 & 1 \\
\end{array}
\right)$
be the transition between the two bases.
Then canonical coordinates are transormed in new coordinates
(with respect to base $\mathcal{F}$ ) by inverse matrix, which is
$N_{\mathcal{F}}=\left(
\begin{array}{ccc}
1 & -1 & 0 \\
0 & 1 & -1 \\
0 & 0 & 1 \\
\end{array}
\right)$.
Take
$A=\left\{a_1,a_2,a_3\right\}$
and get new coordinates
$B=N_{\mathcal{F}}.A$.
Then, with $S=T.M_{\mathcal{F}}$
we see:
$T.A=T.M_{\mathcal{F}}.N_{\mathcal{F}}.A=S.B$.
It's not a miracle, only lin. Algebra.
Key is transformation of basis, which implies
transformation of coordinates. That's all.
By the way: Calculating without inverses is not
possible. Your transformation with bases must be
regular. They must be invertible, otherwise it didn't
work.
Let's see. Other basis
$\mathcal{B}=\left\{2 e_1+5 e_3,e_1+e_2+6 e_3,3 e_1+9 e_3\right\}$,
another transition:
$M_{\mathcal{B}}=\left(
\begin{array}{ccc}
2 & 1 & 3 \\
0 & 1 & 0 \\
5 & 6 & 9 \\
\end{array}
\right)$.
The inverse:
$N_{\mathcal{B}}=\left(
\begin{array}{ccc}
3 & 3 & -1 \\
0 & 1 & 0 \\
-\frac{5}{3} & -\frac{7}{3} & \frac{2}{3} \\
\end{array}
\right)$.
Old transformation T
$T=\left(
\begin{array}{ccc}
3 & 1 & 0 \\
1 & 0 & 1 \\
1 & 0 & -1 \\
\end{array}
\right)$.
Transformed T:
$S=T.M_{\mathcal{B}}=\left(
\begin{array}{ccc}
6 & 4 & 9 \\
7 & 7 & 12 \\
-3 & -5 & -6 \\
\end{array}
\right)$
Transformed A:
$B=N_{\mathcal{B}}.A$.
$T.A=T.M_{\mathcal{B}}.N_{\mathcal{B}}.A=S.B$
Like before.
Best Answer
$$\begin{pmatrix}6\\\!\!-1\\4\end{pmatrix}=a\begin{pmatrix}1\\0\\0\end{pmatrix}+b\begin{pmatrix}2\\2\\0\end{pmatrix}+c\begin{pmatrix}3\\3\\3\end{pmatrix}\iff$$
$$\begin{align*}a+2b+3c&=6\\ 2b+3c&=-1\\ 3c&=4\end{align*}$$
Well, now just find $\,a,b,c\,$ and these will be your coordinates for your vector wrt the given basis. The inverse process you already did, just as John pointed out.